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Fluctuation-Dissipation Framework for Size-Dependent Surface Tension
arXiv:2605.13244v2 Announce Type: replace-cross Abstract: The size-dependent liquid-vapor surface tension controls phase change, wetting, and transport at nanoscales, yet its first curvature correction, the Tolman length, remains difficult to determine. We develop a thermodynamic and statistical-mechanical framework that relates this correction to bulk response properties of a one-component liquid near liquid-vapor coexistence. For curved interfaces, the analysis considers two local...