Size-Dependent CO2 Reduction Selectivity
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Revealing Wavelength- and Size-Dependent CO2 Reduction Selectivity via Operando Scanning Photo-Electrochemical Microscopy
Announce Type: new Abstract: Controlling product selectivity in plasmonic catalysis, particularly in CO2 reduction (CO2R), remains a central unsolved challenge with direct implications for light-driven fuel and chemical synthesis. Here, we deploy quantitative operando scanning photoelectrochemical microscopy (photo-SECM) to provide a direct demonstration that tuning photon energy switches CO2R selectivity through an electronically driven pathway. On plasmonic Au/p-GaN photocathodes,...