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Two-dimensional fluorescence spectroscopy with quantum entangled photons: Idler-referenced timing without pump detection
Announce Type: replace Abstract: Entangled photons have attracted increasing interest as resources for developing time-resolved spectroscopic techniques. Theoretical studies suggest that their non-classical correlations enable time-resolved spectroscopy with monochromatic pumping and can selectively isolate specific Liouville pathways in nonlinear optical signals. In an earlier study, we proposed a fluorescence detection scheme that could, in principle, be implemented using existing...