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Roles of individual pigments in ultrafast excitation dynamics of light-harvesting phycobiliproteins revealed by recombinant techniques and two-dimensional electronic spectroscopy
Announce Type: replace Abstract: Phycobiliproteins serve as highly efficient light-harvesting antennae in cyanobacteria, yet the molecular factors governing their ultrafast energy relaxation and coherence dynamics remain incompletely understood. In this study, we investigate the role of pigment arrangement and pigment-protein interactions by combining recombinant protein engineering with two-dimensional electronic spectroscopy (2D-ES). In addition to wild-type allophycocyanin (APC) and...