Reinforcement Learning Efficient Active Space Engine
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RLEASE: Reinforcement Learning Efficient Active Space Engine
arXiv:2606.07879v1 Announce Type: new Abstract: Selecting the active space for multireference electronic-structure calculations is a long-standing bottleneck that often requires expert chemical intuition and costly trial-and-error. We introduce RLEASE (Reinforcement Learning Efficient Active Space Engine), a low-cost method for automatic, geometry-dependent active-space selection. A neural network predicts per-orbital diagnostic scores ($\hat{s}_{1}$) from inexpensive Hartree-Fock orbital...
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